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1 Huanli Gao -- 159 2026-09-22 15:03:33

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Gao, H. Paper-Based Materials. Encyclopedia. Available online: https://encyclopedia.pub/entry/60268 (accessed on 23 September 2026).
Gao H. Paper-Based Materials. Encyclopedia. Available at: https://encyclopedia.pub/entry/60268. Accessed September 23, 2026.
Gao, Huanli. "Paper-Based Materials" Encyclopedia, https://encyclopedia.pub/entry/60268 (accessed September 23, 2026).
Gao, H. (2026, September 22). Paper-Based Materials. In Encyclopedia. https://encyclopedia.pub/entry/60268
Gao, Huanli. "Paper-Based Materials." Encyclopedia. Web. 22 September, 2026.
Paper-Based Materials
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Paper-based materials are hierarchical composite materials composed primarily of a three-dimensional network of cellulose fibers, frequently supplemented with inorganic fillers, chemical additives, or polymer matrices. The structural integrity of these materials arises from inter-fiber bonding mechanisms, predominantly hydrogen bonding between hydroxyl groups on cellulose surfaces, alongside mechanical interlocking and physical entanglement of the fibrous elements [1]. The formation process involves the dewatering and consolidation of an aqueous fiber suspension, which results in a porous, heterogeneous microstructure characterized by varying degrees of fiber orientation, density gradients, and inter-fiber contact areas [2]. This fibrous architecture imparts distinct physical and mechanical characteristics, including pronounced anisotropy, flexibility, and tunable porosity, which differentiate paper-based materials from monolithic polymers or dense composite systems [3]. The material properties are intrinsically linked to the hierarchical organization of cellulose at multiple length scales, ranging from nanoscale microfibrils and amorphous/crystalline domains within individual fibers to the macroscopic arrangement of the fiber network [3].

cellulose fiber network inter-fiber bonding hierarchical microstructure anisotropic properties

References

  1. C T J Dodson; The nature of bonds in paper and the behaviour of paper under mechanical strain. Rep. Prog. Phys. 1970, 33, 1-43. [CrossRef]
  2. Chisom C. Umeileka; Lucian A. Lucia; Melissa A. Pasquinelli; Martin A. Hubbe; Concepts and evidence of interdigitation in the strength development of paper and sheets formed from highly fibrillated cellulose: A review. BioResources 2026, 21, 5666–5705. [CrossRef]
  3. Mahiar Max Hamedi; Mats Sandberg; Richard T. Olsson; Jan Pedersen; Tobias Benselfelt; Jakob Wohlert; Wood and Cellulose: the Most Sustainable Advanced Materials for Past, Present, and Future Civilizations. Adv. Mater. 2025, 37, e2415787. [CrossRef]
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