Particulate matter emissions from aircraft engines contribute to ambient concentrations of ultrafine particles in and around airports together with other combustion sources including road traffic. The impact of emissions on ambient concentrations from an airport, for which aircraft engine is a main source, differs from airport to airport due to the different relative contributions of other sources such as road traffic, and due to pollutant mix differences, chemical characteristics and size distribution [1,2]. Particulate matter, particularly the ultrafine component made up of small particles with an aerodynamic diameter of less than 0.1 µm, is widely considered a health hazard [3]. Aircraft gas turbine engines result in direct emissions of “non-volatile” (nvPM), also described as black carbon (BC) “soot” emissions. In addition to local air quality impacts, particles emitted from aircraft engines can affect climate and cloudiness in a number of ways [8]. There are several on-going projects such as AVIATOR [9] and ACACIA [10], that are taking measurements, linking these to modelling and assessing the particulate impacts on local air quality and climate.
The combustion technology has had to evolve to control these regulated pollutants in addition to the principal imperatives of safety and operability. In the current engine designs that are now in service, the environmental focus of the combustion design has been controlling NOx emissions whilst improving fuel efficiency. However, as the relevance of nvPM emissions has increased, the design of combustors has to consider both NOx and nvPM emissions as well as fuel efficiency and, of course, all within the safety and operability constraints (altitude relight, turbine inlet temperature, combustion efficiency, combustion instabilities, thermal load, etc.) which bound the main design decisions.
Modern engines designed for subsonic aeroplanes generally tend to easily achieve the CO and unburnt HC emissions regulations; these pollutants are now of such low concentrations that they are no longer considered to be of much concern in urban or around airport locations. The focus of the following sections is to examine the most recent design features of combustors that affect the emissions of nvPM and NOx, which are of most current environmental concern. The two main modern combustion technologies are covered: the most widespread, Rich-burn, Quick-quench, Lean-burn (RQL) and Lean Burn (LB) technologies.
ICAO requires that turbofan engines of maximum rated thrust at sea level greater than 26.7 kN be certified for their emission performance. There are however other classes of engines that do not fall under this regulated category. These non-regulated engines include the following: (i) small turbofan engines with rated thrust below 26.7 kN and often used on business jets and small private jets; (ii) military turbofan engines; (iii) auxiliary power units (APUs); (iv) turboprop engines; (v) turboshaft engines mainly used on helicopters; and (vi) piston (or reciprocating) engines. For these unregulated engines, there are limited publicly available data, exposing a knowledge gap in aviation environmental impact assessment and mitigation. It should be noted that on a global scale, nvPM emissions from non-regulated engines are significantly lower compared to the regulated ones, and on a local scale this is likely to be true around large airports too. However, non-regulated engines may be significant emission sources at airports that mainly service aircraft listed (i) to (vi) above and therefore, could be a concern for the local population around these airports. Here, we present a summary of available data with respect to the emission profiles and emission performance of unregulated engines. Unlike the regulated engines, available data in this case are often not reported according to the ICAO-prescribed LTO cycle.
A summary of the literature on emission profiles from non-regulated engines can be found in Table 1. One main theme is the lack of publicly available data. Where data were available, there is no clear and consistent standardized measurement method or power setting across the different studies. Engine properties for which emissions were measured in some cases are unknown, for instance, APUs. A standardized test program including information allowing for example loss corrections would improve the quality and usability of available data for air quality modelling and development of inventories. In addition to missing engine characteristics, particulate emission data are limited for most engine classes. For military turbofan, turboprop and turboshaft engines, these data are primarily from the 1970s and 1980s; methods applied are relatively outdated.
Studies | Type of Engine | Description of Data | Measured/Reported Compounds | |||||||||||||||||||||
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Durdina et al., 2019 [37] | Durdina et al., 2019 [26] |
Turbofan < 26.7 kN | Measured nvPM emissions from a Dassault 900EX carrying three Honeywell TFE731-60 engines were similar in profile to larger engine measurements. | nvPM mass and number, GMD | ||||||||||||||||||||
Klapmeyer and Marr (2012) [47] | Klapmeyer and Marr (2012) [27] | Turbofan < 26.7 kN | Plume measurements, during regular airport operations, of NO | x | , CO | 2 | , and PM from Cessna C560 aircrafts carrying two Pratt & Whitney (PW) JTD15-5 engines during idle/taxi and at take-off. | NO | x | , Particle number, CO | 2 | |||||||||||||
ICAO EEDB [13] | ICAO EEDB [2] | Turbofan < 26.7 kN | Pratt & Whitney reported emissions from JT15D series (-1, -4, -5, -5A, -5B, -5C) and corrected as prescribed by ICAO. Allied Signal reported emissions from TFE731-2-2B and TF3731-3 engines | Reported on ICAO EEDB; HC, CO, NO | x | , SN | ||||||||||||||||||
Spicer et al., 2009, 1992, 1989, 1987 [40,44,48,49] | Spicer et al., 2009, 1992, 1989, 1987 [28][29][30][31] | Military turbofans | Military turbofan engines have different power modes than non-military turbofan engines including an afterburn power mode. However, excluding afterburn power mode for which emissions data are very scarce, military turbofan engine emission profiles are like other turbofan engines. Particle emissions measured as smoke numbers showed highest smoke numbers at 75% to intermediate power and lowest at idle to 30% of normal rated power. Measured airplane engines include F110, F101, F100-PE-100, TF41-42, TF30-P103, TF30-P109. | (JP-4 fuel; [44]: JP-8 + 100) HC, CO, NO | (JP-4 fuel; [29]: JP-8 + 100) HC, CO, NO | x | , SN | |||||||||||||||||
Bulzan et al., 2010; Crayford and Johnson, 2011; Khandelwal et al., 2019; Kinsey et al., 2012 Lobo et al., 2015 [4,23,38,39,50] | Bulzan et al., 2010; Crayford and Johnson, 2011; Khandelwal et al., 2019; Kinsey et al., 2012 Lobo et al., 2015 [11][17][32][33][34] |
APUs | Generally, APUs show similar CO and HC emission profiles to larger turbofan engines. Observed NO | x | emissions were different; while some studies observed no change in NO | x | emissions, others observed some increase in NO | x emission with increasing power [38,39]. Particle mass EIs decreased with increasing power demand for GTCP85 series [4,23,38], whereas a Rolls Royce Artouste Mk113 APU had higher PM mass concentration (mg/m | emission with increasing power [32][33]. Particle mass EIs decreased with increasing power demand for GTCP85 series [11][17][32], whereas a Rolls Royce Artouste Mk113 APU had higher PM mass concentration (mg/m | 3) at full power than at idle [39]. Lobo et al. (2015) observed lowest PM number EIs at highest power. Kinsey et al.’s (2012) study was inconclusive in PM number EIs as different research groups in the same campaign showed different particle number EI profiles; some were u-shaped with maximum at highest power, others showed no variation with power. For the Kinsey et al.’s group (2012), using Fischer Tropsch fuel (FT; synfuel) reduced PM number and mass EI, and had a clear profile of decreasing EIs with increasing exhaust gas temperature. Crayford et al. observed higher smoke number (SN) and PM number concentrations (number/cm | ) at full power than at idle [33]. Lobo et al. (2015) observed lowest PM number EIs at highest power. Kinsey et al.’s (2012) study was inconclusive in PM number EIs as different research groups in the same campaign showed different particle number EI profiles; some were u-shaped with maximum at highest power, others showed no variation with power. For the Kinsey et al.’s group (2012), using Fischer Tropsch fuel (FT; synfuel) reduced PM number and mass EI, and had a clear profile of decreasing EIs with increasing exhaust gas temperature. Crayford et al. observed higher smoke number (SN) and PM number concentrations (number/cm | 3) at full power than at idle [39]. | ) at full power than at idle [33]. | [38] (JP-8, and FT-2): HC, NO | [32] (JP-8, and FT-2): HC, NO | x, CO, nvPM mass and number [39]: HC, CO, NO | , CO, nvPM mass and number [33]: HC, CO, NO | x, SN [4] (JP-8, and FT-2): SO | , SN [17] (JP-8, and FT-2): SO | 2 | , HC, CO, NO | x, nvPM mass and number [23] (Jet A1): nvPM mass and number [50] (Jet A1): CO and NO | , nvPM mass and number [11] (Jet A1): nvPM mass and number [34] (Jet A1): CO and NO | x |
Cain et al., 2013; Corporan et al., 2007, 2010, 2004; Drozd et al. 2012; Kinsey et al., 2019 [41,42, | [35] | 43, | [36] | 51, | [ | 52,53] | Cain et al., 2013; Corporan et al., 2007, 2010, 2004; Drozd et al. 2012; Kinsey et al., 201937][38][39][40] | Turboshaft engines (primarily used on helicopters) | Variable observations were made for particulate emissions, probably due to differences in sampling methods. There was a general agreement in particle number emissions. Particulate number and mass emissions (concentrations and EIs) and geometric mean diameter (GMD) increased with increasing power. General emission profiles of emissions of CO, NO | x | , and HC are like those of turbofan engines. PM emissions were significantly reduced with FT fuel. | [51] (JP-8): CO | [38] (JP-8): CO | 2, CO, PM mass and number, particle size distribution (PSD) [22,41,43,52,54] (JP-8, FT): GMD, SN, CO, NO | , CO, PM mass and number, particle size distribution (PSD) [10][35][37][39][41] (JP-8, FT): GMD, SN, CO, NO | x, PM mass and number [42] (JP-8, FT): PM mass, CO, CO | , PM mass and number [36] (JP-8, FT): PM mass, CO, CO | 2, HC [53] (JP-8, FT): GMD, CO, CO | , HC [40] (JP-8, FT): GMD, CO, CO | 2 | , HC | |||
Chan et al., 2013; Cheng et al., 2008; Corporan et al., 2008; Spicer et al., 2009 [44,45,54,55] | Chan et al., 2013; Cheng et al., 2008; Corporan et al., 2008; Spicer et al., 2009 [29][41][42][43] |
Turboprop engines (primarily on military aircraft) | Emission measurements were primarily conducted on turboprop engines for military purposes as in the T56 series III engines on C-130 Hercules (C-130H) aircraft. Power in turboprop engines is reported as shaft horsepower (shp). The gaseous emission profiles observed for the T56 series engines are like those of turboshaft engines. Particle number and mass emissions tended to decrease with an increase in power. | [55] (JP-8): CO, NO | [43] (JP-8): CO, NO | x | , CO | 2 | , SO | x [54] (JP-8): SN, PM number and mass, GMD, CO, NO | [41] (JP-8): SN, PM number and mass, GMD, CO, NO | x | , CO | 2 [44] (JP8): CO, NO | [29] (JP8): CO, NO | x, OC [45] (F-34, 50-50 F34/Camelina-HEFA blend): PM number and mass, NO | , OC [42] (F-34, 50-50 F34/Camelina-HEFA blend): PM number and mass, NO | x | , CO, HC |
As the exhaust leaves the engine, the hot combustion exhaust gases cool down and liquid droplets and condensation nuclei of mainly sulphates are formed, on the surfaces of which further substances such as water and organics can condense. Shortly after formation, these particles have typical diameters of a few nanometers. Both the number and mass of particles change significantly during transport due to processes such as agglomeration, condensation, and evaporation on a timescale from seconds to several tens of minutes. An effective emission rate can be derived from the number of particles in the cooled exhaust gas. These particles are referred to as volatile or semi-volatile ultrafine particles but here, the simplified term volatile particulate matter (vPM) is used.
Timko et al. [29][18] report on measurements during the AAFEX campaign. Particles (sum of vPM and nvPM) were measured at distances between 30 m and 300 m behind a CFM56 engine for different power settings and types of fuel. At distances with moderate dilution, as compared to the smaller distance (30 m) from the engine exit, more particles were measured as condensation nuclei were formed in the plume. The study also observed that the nucleation of particles accelerates with increasing fuel sulphur content, as these new particles are generated largely from sulphates. About one order of magnitude more particles were observed for low power while the difference was less pronounced for higher powers. The autscholars deduce that the PM evolution strongly depends on the ratio of particle precursors (sulphate and organics) to soot; more nvPM particles are generated at higher powers and lead to a greater interaction between precursors and nvPM with more coating of nvPM with sulphuric acid, etc. and thereby to a smaller total number of newly formed particles as compared to lower powers.
An emission inventory typically comprises a dataset with emission amounts, in terms of mass, for the most relevant air pollutant and greenhouse gas species, split up by source type, time and location. Different levels of spatial and temporal resolution are possible, depending on the scope and purpose of the inventory. Aircraft emissions inventories usually report only those emissions related to the LTO cycle for the aircraft, which covers activities up to 3000 feet (914 m), which coincides with the typical order of magnitude for the height of the neutrally stratified atmospheric mixing layer. Emissions below this altitude are expected to be the dominant influence for local ground-level air quality parameters. The 3000 feet boundary is also used as the cut-off altitude for reporting national emissions for air pollution under EMEP (Gothenburg Protocol) and the EU National Emission Ceilings Directive (2016/2284/EU), so national emission inventories often pay limited attention to what happens at higher altitudes.